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  • 05월 20일 18시 이후 : 초록수정 불가능, 일정확인 및 검색만 가능

제125회 대한화학회 학술발표회 및 총회 Stimulated Raman spectroscopy for characterizing two-dimensional crystals

등록일
2020년 2월 3일 13시 58분 02초
접수번호
0177
발표코드
PHYS.P-215 이곳을 클릭하시면 발표코드에 대한 설명을 보실 수 있습니다.
발표시간
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발표형식
포스터
발표분야
Physical Chemistry
저자 및
공동저자
Hwansoo Jeon, Sunmin Ryu*
Department of Chemistry, Pohang University of Science and Technology, Korea
Two-dimensional dielectric materials such as hexagonal BN and mica give very weak signals in conventional spontaneous Raman scattering using visible excitation lasers. In this work, we report a micro-spectroscopy setup for stimulated Raman scattering (SRS), which gives a substantial increase in overall sensitivity. Pump and Stokes beams with temporal width of a few ps were prepared by spectrally slicing 200 fs pulses from an optical parametric oscillator. The pulse slicer acting as a narrow band-pass filter consisted of a grating (1200 grooves/mm), a cylindrical lens, a mirror, and a mechanical slit that were arranged in the 4f-configuration. Whereas the Stokes pulses were fixed at 1040 nm with a bandwidth of 0.7 nm, the pump pulses were varied from 734 nm to 998 nm for the Raman shift in the range of 400 ~ 4000 cm-1. The pump beam modulated by interaction with the Stokes beam was measured using an in-line balanced detection method with photodiodes that were connected to a lock-in amplifier. The sensitivity of the SRS method will be presented with technical details of the setup.

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